ABSTRACT
The lockdown in 2020 implemented due to the SARS-CoV-2 pandemic has resulted in a significant improvement in air quality at a global scale. Nationwide lockdown also considerably improved air quality at a local scale, especially in cities which were almost completely shut down during the first coronavirus wave, with nearly no activity. We tested the hypothesis that a reduction in the intensity of vehicle traffic causes a drastic decrease in urban air pollution at a local scale. We focused on two urban agglomerations, Warsaw and Cracow, in Poland. Data of the concentrations of traffic-related sources, namely NOx, PM10, and PM2.5, obtained from two air pollution monitoring stations were analyzed for the years 2020 and 2021, during which lockdown and pandemic restrictions were in effect, and for 2019, as a reference. In the years 2020–2021, the average annual concentration of NOx was decreased by ~ 19%, PM2.5 by ~ 19%, and PM10 by ~ 18% in Warsaw, while in Cracow the average annual concentration of NOx was decreased by ~ 16%, PM2.5 by ~ 22%, and PM10 by ~ 2%, compared to 2019. The contribution from traffic-related sources to the overall level of air pollution was estimated. The results indicated that ~ 30 µg/m3 of PM10, ~ 15 µg/m3 of PM2.5, and ~ 120 µg/m3 of NOx in Cracow, and ~ 20 µg/m3 of PM2.5 in Warsaw originate from moving vehicles. The nationwide lockdown allowed us to conduct this study to understand how a reduction in local traffic emissions can decrease ambient air pollution levels.
ABSTRACT
A knowledge gap exists concerning how chemical composition and sources respond to implemented policy control measures for aerosols, particularly in a semi-arid region. To address this, a single year's offline measurement was conducted in Hohhot, a semi-arid city in northern China, to reveal the driving factors of severe air pollution in a semi-arid region and assess the impact of the COVID-19 lockdown measures on chemical characteristics and sources of PM2.5. Organic matter, mineral dust, sulfate and nitrate accounted for 31.5 %, 14.2 %, 13.4 % and 12.3 % of the total PM2.5 mass, respectively. Coal combustion, vehicular emission, crustal source and secondary inorganic aerosols were the main sources of PM2.5 in Hohhot, at 38.3 %, 35.0 %, 13.5 %, and 11.4 %, respectively. Due to the coupling effect of emission reduction and improved atmospheric conditions, the concentration of secondary inorganic components, organic matter and elemental carbon declined substantially from the pre-lockdown (pre-LD) period to the lockdown (LD) and post-lockdown (post-LD) periods. The source contribution of secondary inorganic aerosols increased (from 21.1 % to 37.8 %), whereas the contribution of vehicular emission reduced (from 35.5 % to 4.4 %) due to lockdown measures. The rapid generation of secondary inorganic components caused by unfavorable meteorological conditions during lockdown led to serious pollution. This study elucidates the complex relationship between air quality and environmental policy.
ABSTRACT
To control the spread of COVID-19, exceptional restrictive measures were taken in March 2020 that imposed a radical change on the lifestyle of millions of citizens around the world, albeit for a short period. The national lockdown, which lasted from 10 March to 18 May 2020 in Italy, was a unique opportunity to observe the variation in air quality in urban environments under conditions comprising almost total traffic restriction and a strong reduction in work activities. In this paper, the data from 17 urban monitoring sites in Tuscany are presented, and the PM and NO2 concentrations in the 2 months before the start of the lockdown and the 2 months after lockdown are compared with the corresponding months of the previous 3 years. The results show that the total loads of PM2.5 and PM10 (particulate matter with an aerodynamic diameter smaller than 2.5 and 10 µm, respectively) decreased, but they did not exhibit significant changes compared to previous years, whereas NO2 underwent a drastic reduction. For three of these sites, the chemical composition of the collected samples was measured using thermal–optical techniques, ion chromatography, and particle-induced X-ray emission analysis, and the application of multivariate positive matrix factorization analysis also allowed for PM10 source identification and apportionment. Using these analyses, it was possible to explain the low sensitivity of PM10 to the lockdown effects as being due to different, sometimes inverse, behaviors of the different sources that contribute to PM. The results clearly indicate a decline in pollution levels related to urban traffic and an increase in the concentration of sulfate for all sites during the lockdown period.
ABSTRACT
Previous studies have determined biomass burning as a major source of air pollutants in the ambient air in Thailand. To analyse the impacts of meteorological parameters on the variation of carbonaceous aerosols and water-soluble ionic species (WSIS), numerous statistical models, including a source apportionment analysis with the assistance of principal component analysis (PCA), hierarchical cluster analysis (HCA), and artificial neural networks (ANNs), were employed in this study. A total of 191 sets of PM2.5 samples were collected from the three monitoring stations in Chiang-Mai, Bangkok, and Phuket from July 2020 to June 2021. Hotspot numbers and other meteorological parameters were obtained using NOAA-20 weather satellites coupled with the Global Land Data Assimilation System. Although PCA revealed that crop residue burning and wildfires are the two main sources of PM2.5, ANNs highlighted the importance of wet deposition as the main depletion mechanism of particulate WSIS and carbonaceous aerosols. Additionally, Mg2+ and Ca2+ were deeply connected with albedo, plausibly owing to their strong hygroscopicity as the CCNs responsible for cloud formation.
ABSTRACT
Based on monitoring data of atmospheric pollutants in Nanjing from Jan. 1, 2015 to Feb. 10, 2021, the spatial-temporal distribution characteristics of Nanjing's ambient air quality and the contribution of potential source areas were analyzed. The average concentrations of six air pollutants (CO, NO2 , SO2 , O3, PM10, and PM2.5) were 800 µg. m-3, 43. 1 µg . m-3, 13. 0 µg . m-3, 106. 0 µg . m-3, 77. 1 µg . m-3, and 43. 0µg . m-3, respectively. The average concentration of ozone in Nanjing was higher than that in China's other typical cities (Beijing, Shanghai, Guangzho, Chengd, Lanzhou, and Wuhan). The number of pollution days for NO2,PMl0,and PM2.5 were reduced by 29. 1% ,38. 1% ,and 28. 1% during 2015 to 2020. However, the frequency of ozone pollution days was increasing (the highest value in summer and the lowest value in winter). The potential source analysis of fine particulate matter in January of 2015-2020 was carried out. It was found that the potential source for Nanjing's PM2.5 was surrounding industrial areas (Anhui province,north of Jiangsu province, and Shandong province). The concentration of air pollutants in Nanjing in 2020 was lower than that in 2019 and 2021. It indicated that the reduction of human activity caused by COVID-19 pandemic has resulted in less air pollutant emissions and improved air quality in Nanjing.
ABSTRACT
A powerful methodology, based on the multivariate curve resolution alternating least squares (MCR-ALS) method with quadrilinearity constraints, is proposed to handle complex and incomplete four-way atmospheric data sets, providing concise results that are easy to interpret. Changes in air quality by nitrogen dioxide (NO2), ozone (O3), and particulate matter (PM10) in eight sampling stations located in the Barcelona metropolitan area and other parts of Catalonia during the COVID-19 lockdown period (2020) with respect to previous years (2018 and 2019), are investigated using such methodology. The MCR-ALS simultaneous analysis of the three contaminants among the eight stations and for the 3 years allows the evaluation of potential correlations among the pollutants, even when having missing data blocks. Correlated profiles are shown by NO2 and PM10 due to similar pollution sources (traffic and industry), evidencing a decrease in 2019 and 2020 due to traffic restriction policies and the COVID-19 lockdown period, especially noticeable in the most transited urban areas (i.e., Vall d'Hebron, Granollers and Gràcia). The O3 evidences an opposed interannual trend, showing higher amounts in 2019 and 2020 with respect to 2018 due to the decreased titration effect, more significant in rural areas (Begur) and in the control site (Obserbatori Fabra).
ABSTRACT
PM2.5 concentrations in urban areas are highly variable, both spatially and seasonally. To assess these patterns and the underlying sources, we conducted PM2.5 exposure measurements at the adult breath level (1.6 m) along three ~5 km routes in urban districts of Mainz (Germany) using portable low-cost Alphasense OPC-N3 sensors. The survey took place on five consecutive days including four runs each day (38 in total) in September 2020 and March 2021. While the between-sensor accuracy was tested to be good (R² = 0.98), the recorded PM2.5 values underestimated the official measurement station data by up to 25 µg/m3. The collected data showed no consistent PM2.5 hotspots between September and March. Whereas during the fall, the pedestrian and park areas appeared as hotspots in >60% of the runs, construction sites and a bridge with high traffic intensity stuck out in spring. We considered PM2.5/PM10 ratios to assign anthropogenic emission sources with high apportionment of PM2.5 in PM10 (>0.6), except for the parks (0.24) where fine particles likely originated from unpaved surfaces. The spatial PM2.5 apportionment in PM10 increased from September (0.56) to March (0.76) because of a pronounced cooler thermal inversion accumulating fine particles near ground. Our results showed that highly resolved low-cost measurements can help to identify PM2.5 hotspots and be used to differentiate types of particle sources via PM2.5/PM10 ratios.
ABSTRACT
This review provides a community's perspective on air quality research focusing mainly on developments over the past decade. The article provides perspectives on current and future challenges as well as research needs for selected key topics. While this paper is not an exhaustive review of all research areas in the field of air quality, we have selected key topics that we feel are important from air quality research and policy perspectives. After providing a short historical overview, this review focuses on improvements in characterizing sources and emissions of air pollution, new air quality observations and instrumentation, advances in air quality prediction and forecasting, understanding interactions of air quality with meteorology and climate, exposure and health assessment, and air quality management and policy. In conducting the review, specific objectives were (i) to address current developments that push the boundaries of air quality research forward, (ii) to highlight the emerging prominent gaps of knowledge in air quality research, and (iii) to make recommendations to guide the direction for future research within the wider community. This review also identifies areas of particular importance for air quality policy. The original concept of this review was borne at the International Conference on Air Quality 2020 (held online due to the COVID 19 restrictions during 18–26 May 2020), but the article incorporates a wider landscape of research literature within the field of air quality science. On air pollution emissions the review highlights, in particular, the need to reduce uncertainties in emissions from diffuse sources, particulate matter chemical components, shipping emissions, and the importance of considering both indoor and outdoor sources. There is a growing need to have integrated air pollution and related observations from both ground-based and remote sensing instruments, including in particular those on satellites. The research should also capitalize on the growing area of low-cost sensors, while ensuring a quality of the measurements which are regulated by guidelines. Connecting various physical scales in air quality modelling is still a continual issue, with cities being affected by air pollution gradients at local scales and by long-range transport. At the same time, one should allow for the impacts from climate change on a longer timescale. Earth system modelling offers considerable potential by providing a consistent framework for treating scales and processes, especially where there are significant feedbacks, such as those related to aerosols, chemistry, and meteorology. Assessment of exposure to air pollution should consider the impacts of both indoor and outdoor emissions, as well as application of more sophisticated, dynamic modelling approaches to predict concentrations of air pollutants in both environments. With particulate matter being one of the most important pollutants for health, research is indicating the urgent need to understand, in particular, the role of particle number and chemical components in terms of health impact, which in turn requires improved emission inventories and models for predicting high-resolution distributions of these metrics over cities. The review also examines how air pollution management needs to adapt to the above-mentioned new challenges and briefly considers the implications from the COVID-19 pandemic for air quality. Finally, we provide recommendations for air quality research and support for policy.